• Overture — Orchestral medley pada beberapa lagu dari filem, termasuk "Feed the Birds", "A Spoonful of Sugar", "Chim Chim Cher-ee" dan "Supercalifragilisticexpialidocious".
• "Jolly Holiday" — A few bars of the song, dimainkan oleh Dick Van Dyke dengan perkakas "one man band"nya.
• "Sister Suffragette" — Dick Van Dyke, Glynis Johns, Hermione Baddeley dan Reta Shaw, dengan gangguan bukan-bernyanyi oleh Elsa Lanchester. Secara asas didengari dalam suatu rendisi a cappella oleh Johns, hanya sebelum nyanyian yang penuh, lagu ditemani-orkestra dengan para pekerja rumah; dan suatu versi muzik sahaja dalam langkah "Step in Time".
• "The Life I Lead" — David Tomlinson (kemudian dibalas dengan Julie Andrews sebagai "A British Bank".)
• "The Perfect Nanny" — Karen Dotrice dan Matthew Garber
• "A Spoonful of Sugar" — Julie Andrews (pembebasan DVD 2004 mendedahkan bahawa Andrews juga mempersembahkan siulan burung swaktu nombor ini)
• "Jolly Holiday" — Dick Van Dyke dan Julie Andrews, dengan Thurl Ravenscroft, Marni Nixon, Paul Frees dan yang lain
• "Supercalifragilisticexpialidocious" — Julie Andrews dan Dick Van Dyke dengan J. Pat O'Malley dan yang lain
• "Stay Awake" — Julie Andrews
• "I Love to Laugh" — Dick Van Dyke, Julie Andrews dan Ed Wynn
• "Feed the Birds" — Julie Andrews (lagu kegemaran Walt Disney dari skor, dan melodi leadoff dalam percubaan memulakan suatu hubungan)
• "Fidelity Fiduciary Bank" — Dick Van Dyke, David Tomlinson dan yang lain
• "Chim Chim Cher-ee" — Dipersembahkan banyak kali dengan lirik berlainan dengan Dick Van Dyke; juga dipersembahkan oleh Van Dyke dengan Julie Andrews, Karen Dotrice, dan Matthew Garber (memenangi Academy Award untuk Best Original Song)
• "Step in Time" — Dick Van Dyke
• "A Man Has Dreams" — David Tomlinson dan Dick Van Dyke. Rendisi langkah yang lebih berpelahan-lahan pada "The Life I Lead" yang menggubahkan versi dimodifikasikan "A Spoonful of Sugar".
• "Feed the Birds" — Balasan orchestral dan choral, dimainkan ke atas jalan sendirian Mr. Banks ke bank pada waktu malam.
• "Let's Go Fly a Kite" — Glynis Johns, David Tomlinson, Dick Van Dyke dan yang lain.
• Closing credits theme — Termasuk suatu balasan berinstrumen "Spoonful of Sugar" diikuti oleh suatu balasan berkenaan koir "Let's Go Fly a Kite".

Pada 2004, "Supercalifragilisticexpialidocious" telah ditempatkan #36 dalam senarai American Film Institute pada 100 Greatest Songs in Movie History.

Lagu yang dialih

Sebilangan lagu lain dikarang untuk filem oleh Sherman Brothers dan sama ada ditolak atau dipotong oleh kerana waktu. Richard Sherman, dalam pembebasan DVD 2004, menandakan bahawa lebih daripada 30 lagu telah dikarangkan di pelbagai tahap perkembangan filem. Tiada rakaman lakonan pada mana-mana lagu ini telah dibebaskan ke orang ramai, hanya demo atau persembahan kemudiannya dilakukan oleh pengarang lagu — dengan pengecualian reprise atas bumbung "Chim-Chim-Cheree" dan "smoke staircase yodel" disebut di bawah.

• "The Chimpanzoo", was originally to follow "I Love to Laugh" during the Uncle Albert "ceiling tea party" sequence, but it was dropped from the soundtrack just before Julie Andrews and company were to record it. The fast-paced number was not unveiled to the public until Richard Sherman, aided by recently uncovered storyboards, performed it on the 2004 DVD edition. The re-creation suggests it was to have been another sequence combining animation and live action.
• "Practically Perfect" was intended to introduce Mary but instead the melody of the piece was used for "Sister Suffragette" (used to introduce Winifred (Mrs. Banks)). A different song with the same name was written for the stage musical.
• "The Eyes of Love", a romantic ballad, was intended for Bert and Mary, but according to Richard Sherman, Julie Andrews suggested privately to Disney that this song was not suitable. In response, "A Spoonful of Sugar" was written.
• "Mary Poppins Melody" was to be performed when Mary introduces herself to the children. Elements of the song later became part of "Stay Awake". The melody was the basis for a couple of other songs that were ultimately cut from the film.
• "A Name's a Name". Heard on a recording taken of a meeting between the Sherman Brothers and P.L. Travers, this song was originally intended for the nursery scene that later became "A Spoonful of Sugar." The melody was reused for "Mary Poppins Melody".
• "You Think, You Blink" was a short piece that Bert was to sing just before entering the chalk painting (and starting the "Jolly Holiday" sequence). In the film, Dick Van Dyke simply recites the lyric instead of singing it.
• "West Wind" was a short ballad to be sung by Mary. The song was later retitled "Mon Amour Perdu" and used in the later Disney film, Big Red.
• "The Right Side" was to be sung by Mary to Michael Banks after he gets out of bed cranky. It was recycled for the Disney Channel television series, Welcome to Pooh Corner as Winnie the Pooh's personal theme song.
• "Measure Up" was to accompany the scene in which Mary takes the tape measure to Jane and Michael.
• "Admiral Boom" was to be the theme song for the cannon-firing neighbor of the Banks Residence, but it was cut by Walt Disney as being unnecessary. The melody of the song remains in the film, and the bombastic theme is heard whenever Boom appears onscreen. One line from this song ("The whole world takes its time from Greenwich, but Greenwich, they say, takes its time from Admiral Boom!") is spoken by Bert early in the film.
• "Sticks, Paper and Strings" was an early version of "Let's Go Fly a Kite."
• "Lead the Righteous Life", an intentionally poorly-written hymn, was to have been sung by Katie Nanna (Elsa Lanchester) along with Jane and Michael prior to Mary Poppins' arrival. The melody was later reused for a similar song in The Happiest Millionaire
• "The Pearly Song" was not deleted per se but was instead incorporated into "Supercalifragilisticexpialidocious".

The Compass Sequence, a precursor to "Jolly Holiday", was to be a multiple-song sequence. A number of possible musical components have been identified:

• "South Sea Island Symphony"
• "Chinese Festival Song"
• "Tim-buc-too" — elements of this were reused for "The Chimpanzoo" which was also cut
• "Tiki Town" — the melody was reused for "The Chimpanzoo"
• "North Pole Polka"
• "Land of Sand" — later rewritten as "Trust in Me" for the animated version of The Jungle Book
• "The Beautiful Briny" — later used in Bedknobs and Broomsticks
• "East is East" — another variation on the unused "Mary Poppins Melody".

Skor dan muzik yang dialihkan

• Langkah "Step in Time" berakhir dengan sapuan cerobong berselerak oleh suatu serangan hebat bunga paoi ditembak dari rumah Admiral Boom. Dalam bahagian terakhir filem, babak ini dimainkan dengan kesan nada suara dan tiada muzik. Pelepasan DVD termasuk versi asal pada babak yang ditemani oleh suatu susunan muzikal berinstrumen kompleks yang menggabungkan "Step in Time", melodi "Admiral Boom" (lihat diatas), dan "A Spoonful of Sugar". Gubahan muzikal ini dapat didengari dalam runut bunyi asal filem.
• Andrews merakamkan suatu balasan ringkas "Chim-Chim-Cheree" yang ditemani oleh Mary, Bert, dan kanak-kanak apabila mereka berkawat di sepanjang atas bumbung London (suatu balasan berinstrumen "A Spoonful of Sugar" telah digunakan sebagai suatu perarakan pula; meskipun, Andrews dan Dick Van Dyke masih dapat dilihat dan didengar menyanyi balasan "Chim-Chim-Cheree" pada langkah itu, hanya sebelum penyapu cerobong lain bermuncul untuk nombor "Step in Time").
• Burung robin yang Mary Poppins bersiul dengan dalam "A Spoonful of Sugar" terdahulunya menyanyikan suatu lirik juga.
• Andrews juga merakam suatu yodel ringkas yang memecah ke adalam barisan pertama "A Spoonful of Sugar" yang telah digunakan untuk "mengaktifkan" tangga merokok sebelum nombor "Step in Time". Walaupun dikeluarkan dari filem, bahagian filem pada Andrews mempersembahkan ini wujud dan telah dimasukkan dalam DVD 2004. DVD juga mengindikasikan bahawa versi bersilih ganti pada yodel dipersembahkan oleh Dick Van Dyke mungkin juga wujud.